92 1001
Eric Foerster (Eric.Foerster@kit.edu)
Institute of Meteorology and Climate Research (IMK), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe, P.O. Box 3640, Germany
1 | HALO | HKMS | VOC data measured with instrument HKMS (HALO Karlsruher Mass Spectrometer) a Proton Transfer Reaction - Mass Spectrometer onboard the research aircraft HALO
EM-AS-12
1 1
2018 04 03 2022 05 02
0
Time; seconds after midnight (UTC); [s]
25
1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1
-9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999 -9999
FOR; Formaldehyde, volume mixing ratio; [pptV]; quantified by signal integration on protonated FOR (m/z = 31)
FOR_prec; Formaldehyde, precision; [pptV];
FOR_lod; Formaldehyde, humidity dependent in-flight detection limit; [pptV];
MET; Methanol, volume mixing ratio; [pptV]; quantified by signal integration on protonated MET (m/z = 33.2)
MET_prec; Methanol, precision; [pptV];
MET_lod; Methanol, humidity dependent in-flight detection limit; [pptV];
ACN; Acetonitrile, volume mixing ratio; [pptV]; quantified by signal integration on protonated ACN (m/z = 42)
ACN_prec; Acetonitrile, precision; [pptV];
ACA; Acetaldehyde, volume mixing ratio; [pptV]; quantified by signal integration on protonated ACA (m/z = 45)
ACA_prec; Acetaldehyde, precision; [pptV];
ACE; Acetone, volume mixing ratio; [pptV]; quantified by signal integration on protonated ACE (m/z = 59)
ACE_prec; Acetone, precision; [pptV];
ISO; Isoprene, volume mixing ratio; [pptV]; quantified by signal integration on protonated ISO (m/z = 69)
ISO_prec; Isoprene, precision; [pptV];
MVK; Methyl Vinyl Ketone, volume mixing ratio; [pptV]; quantified by signal integration on protonated MVK (m/z = 71)
MVK_prec; Methyl Vinyl Ketone, precision; [pptV];
MEK; Methyl Ethyl Ketone, volume mixing ratio; [pptV]; quantified by signal integration on protonated MEK (m/z = 73)
MEK_prec; Methyl Ethyl Ketone, precision; [pptV];
MEK_lod; Methyl Ethyl Ketone, humidity dependent in-flight detection limit; [pptV];
BEN; Benzene, volume mixing ratio; [pptV]; quantified by signal integration on protonated BEN (m/z = 79)
BEN_prec; Benzene, precision; [pptV];
TOL; Toluene, volume mixing ratio; [pptV]; quantified by signal integration on protonated TOL (m/z = 93)
TOL_prec; Toluene, precision; [pptV];
XYL; Xylene, volume mixing ratio; [pptV]; quantified by signal integration on protonated XYL (m/z = 107)
XYL_prec; Xylene, precision; [pptV];
12
Gas standard used for calibrations: Apel-Riemer, 2016, VOCs in synthetic air with an uncertainty of +/- 5 percent.
VOCs included in the standard: FOR, MET, ACN, ACA, ACE, DMS, ISO, MVK, MEK, BEN, TOL, XYL, Pinene.
VOC concentrations in the standard [ppbV]: 1040.3, 476.9, 514.9, 494, 483.4, 488.6, 486.3, 450.1, 512.1, 494.6, 491, 478.2, 494.1, respectively.
Compounds sensitivities obtained by detecting the respective ion count rate (counts per seconds) in gas standard dilution series.
Determination of volume mixing ratios by normalization (VMR) of ion count rates with interpolated sensitivities of several calibration experiments during the campaign.
Instruments background determined from linearly interpolated blank measurements (approx. every 30 min for 5 minutes - flagged as VMISS) and subtracted from measurement signal.
Exception for FOR, MET, DMS, MEK, BEN, TOL and XYL to previous line: Humidity dependent background determined from exponential (y = a*exp(b*x) + c*x.^d, y - background, x - humidity) or quadratic fit (y = p1*x^2 + p2*x + p3) and subtracted from measurement signal.
However, only applied to BEN, TOL and XYL if correlation coeff of background and humidity > 0.6.
From Background subtraction resulting negative values (in case of very low atmospheric concentrations below LOD) are set to VMISS.
Precision is the statistical noise of ion count rates given in columns VOC_prec.
For calibration a re-filled 2 liter bottle of the parent Apel-Riemer gas standard was used.
Filling of this 2 liter gas standard bottle caused a concentration drift of FOR and MET over time and was corrected.
41
Accuracy is affected by 5 percent uncertainty of the respective mixing ratio in the calibration gas standard plus X percent from the calibration process itself, humidity correction and - if existing - bottle drift correction (errors in X added by Gaussian error propagation).
Total relative accuracies [%] are given in the next lines for each VOC:
FOR_acc: 25
MET_acc: 11
ACN_acc: 7
ACA_acc: 9
ACE_acc: 8
ISO_acc: 7
MVK_acc: 8
MEK_acc: 7
BEN_acc: 8
TOL_acc: 8
XYL_acc: 8
The following lines contain the instrument detection limits given in the units of the respective VOC column.
Additionally, complete humidity dependent in-flight LODs for FOR, MET, DMS and MEK (if available) are given in the columns with VNAME "*_lod".
LODs determined in long laboratory measurements.
FOR_LOD: 186
MET_LOD: 639
ACN_LOD: 22
ACA_LOD: 72
ACE_LOD: 28
ISO_LOD: 25
MVK_LOD: 13
MEK_LOD: 18
BEN_LOD: 15
TOL_LOD: 17
XYL_LOD: 23
Temporal resolution per VOC is ca. 1/67 Hz.
FileName: EMERGE-Asia-12_2018-04-03_HKMS_11VOCs_V06.ames
Version: V06
ChangeLog1: V01->V02: 20190503, Updated humidity correction, calculation of precision and accuracy; Applied bottle drift correction for MET and FOR; Applied humidity dependent background subtraction of FOR; Added VOC dependent LODs.
ChangeLog2: V02->V03: 20191114, Background subtraction now after calculation of VMR; background mask enlarged to +/- 2 mass measurements (~10 s) to neglect switching from sample line <-> background line; values below zero (due to background subtraction) now set to zero (VMISS in V03); update of precision and accuracy.
ChangeLog3: V03->V04: 20200304, 1. Applied humidity (hum) dependent background (bgnd) handling of BEN, TOL, XYL, if correlation coeff of bgnd and hum > 0.6: Means of the 5-minute bgnd measurements are fitted against respective 5-minute means of hum (H3O+(H2O) water cluster on m/z = m37). Hum dependent, smoothed (Savitzky-Golay) bgnd signal calculated from fitted curve and subtracted from measurement signal.
ChangeLog3: V03->V04: 20200304, 2. Procedure of 1. is also applied to MET, but only using all bgnd measurements instead of means.
ChangeLog3: V03->V04: 20200304, 3. In this Version, also conservative in-flight detection limits are added. Furthermore, the laboratory LODs are still included. As the humdity has also an influence on the LOD of FOR and MET, for these two VOCs separate columns with LODs are added.
ChangeLog4: V04->V05: 20201027, 1. All calibrations, instrumental background subtractions and detections limits were improved and/or updated. This can slightly change the VOC concentrations.
ChangeLog4: V04->V05: 20201027, 2. Added MVK (Methyl Vinyl Ketone), MEK (Methyl Ethyl Ketone) and DMS (Dimethylsulfid) for some flights. See VNAME if available in this flight. Backgrounds of MEK and DMS are highly humidity dependent and thus adjusted according to same procedure as formaldehyde. Consider MEK and DMS as preliminary data with still unknown effects concerning background and humidity.
ChangeLog5: V05->V06: 20220502, Formaldehyde (FOR) was reanalyzed and updated. Instrumental background subtraction slightly adjusted, especially for benzene (BEN) and toluene (TOL). Expect minimal changes of VMRs (for BEN and TOL mostly small enlargements).
Data status is final.
[s]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]	[pptV]
Time	FOR	FOR_prec	FOR_lod	MET	MET_prec	MET_lod	ACN	ACN_prec	ACA	ACA_prec	ACE	ACE_prec	ISO	ISO_prec	MVK	MVK_prec	MEK	MEK_prec	MEK_lod	BEN	BEN_prec	TOL	TOL_prec	XYL	XYL_prec
1586	4854	481	1272	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1592	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1598	-9999	-9999	-9999	-9999	-9999	-9999	203	25	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1602	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1403	78	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1607	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1887	54	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1612	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	103	30	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1618	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	104	18	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1624	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	2657	91	213	-9999	-9999	-9999	-9999	-9999	-9999
1631	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	204	26	-9999	-9999	-9999	-9999
1639	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	161	29	-9999	-9999
1645	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1652	2504	453	1268	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1658	-9999	-9999	-9999	1628	314	914	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1664	-9999	-9999	-9999	-9999	-9999	-9999	134	22	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1668	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	906	72	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1674	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1187	45	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1679	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	110	30	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1685	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	239	22	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1691	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	2261	88	215	-9999	-9999	-9999	-9999	-9999	-9999
1698	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	150	24	-9999	-9999	-9999	-9999
1705	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	103	27	-9999	-9999
1711	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	20	26
1719	2613	455	1270	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1725	-9999	-9999	-9999	835	309	912	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1731	-9999	-9999	-9999	-9999	-9999	-9999	109	21	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1735	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	627	67	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1740	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1246	46	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1745	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	37	27	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1751	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	107	18	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1757	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	2034	87	217	-9999	-9999	-9999	-9999	-9999	-9999
1764	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	218	26	-9999	-9999	-9999	-9999
1772	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	290	32	-9999	-9999
1778	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	85	28
1785	1661	447	1281	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1791	-9999	-9999	-9999	3194	323	914	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1797	-9999	-9999	-9999	-9999	-9999	-9999	133	22	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1801	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1151	75	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1807	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	2282	59	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1812	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	51	28	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1818	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	63	17	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1824	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1110	82	222	-9999	-9999	-9999	-9999	-9999	-9999
1831	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	147	24	-9999	-9999	-9999	-9999
1838	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	233	31	-9999	-9999
1844	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	71	28
1852	2784	459	1277	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1858	-9999	-9999	-9999	2195	320	921	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1864	-9999	-9999	-9999	-9999	-9999	-9999	112	21	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1868	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	718	69	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1873	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1353	48	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1878	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	28	27	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1884	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	31	16	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1890	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	728	77	215	-9999	-9999	-9999	-9999	-9999	-9999
1897	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	154	24	-9999	-9999	-9999	-9999
1905	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	150	29	-9999	-9999
1911	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	49	27
1918	3115	462	1274	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1924	-9999	-9999	-9999	2668	323	922	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1930	-9999	-9999	-9999	-9999	-9999	-9999	103	21	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1934	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	820	71	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1940	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1418	49	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1945	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	33	27	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1951	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	76	17	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1957	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1307	82	215	-9999	-9999	-9999	-9999	-9999	-9999
1964	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	192	26	-9999	-9999	-9999	-9999
1971	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	660	40	-9999	-9999
1977	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	123	30
1985	3812	486	1322	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1991	-9999	-9999	-9999	3652	328	923	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
1997	-9999	-9999	-9999	-9999	-9999	-9999	118	21	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
2001	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1031	74	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
2006	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	1464	49	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
2011	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	89	30	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
2017	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	113	19	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999	-9999
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